Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China

W. Xu;X. S. Luo;Y. P. Pan;L. Zhang;A. H. Tang;健林 沈;Y. Zhang;K. H. Li;Q. H. Wu;D. W. Yang;Y. Y. Zhang;吉全 薛;W. Q. Li;Q. Q. Li;L. Tang;S. H. Lu;T. Liang;延安 同;P. Liu;Q. Zhang;正琴 熊;孝均 石;良欢 吴;W. Q. Shi;K. Tian;X. H. Zhong;K. Shi;Q. Y. Tang;L. J. Zhang;J. L. Huang;C. E. He;F. H. Kuang;波 朱;H. Liu;X. Jin;Y. J. Xin;X. K. Shi;E. Z. Du;A. J. Dore;S. Tang;J. L. Collett;K. Goulding;Y. X. Sun;J. Ren;福锁 张;学军 刘

China Agricultural University;Henan Academy of Agricultural Sciences;Institute of Atmospheric Physics Chinese Academy of Sciences;Peking University;China Association for Science and Technology;Beijing Forestry University;Xinjiang Institute of Ecology and Geography; Chinese Academy of Science;Fujian Institute of Tobacco Agricultural Sciences;Yunnan Agricultural University;Sichuan Academy of Agricultural Sciences;Northwest AandF University;Shanxi Academy of Agricultural Sciences;Chinese Academy of Tropical Agriculture Sciences;Guangdong Academy of Agricultural Sciences;Dalian Jiaotong University;Hunan Agricultural University;Hebei Agricultural University;Huazhong Agricultural University;Institute of Mountain Hazards and Environment Chinese Academy of Sciences;Xinjiang Academy of Agricultural Sciences;Qinghai Meteorological Bureau;Forestry and Water Department of Changdao County;Beijing Normal University;NERC Centre for Ecology and Hydrology;Colorado State University;Rothamsted Research;Anhui Academy of Agricultural Sciences;Jilin Academy of Agricultural Sciences

发表时间:2015-11-9

期 刊:Atmospheric Chemistry and Physics

语 言:English

U R L: http://www.scopus.com/inward/record.url?scp=84946781079&partnerID=8YFLogxK

摘要

A Nationwide Nitrogen Deposition Monitoring Network (NNDMN) containing 43 monitoring sites was established in China to measure gaseous NH3, NO2, and HNO3 and particulate NH4+ and NO3- in air and/or precipitation from 2010 to 2014. Wet/bulk deposition fluxes of Nr species were collected by precipitation gauge method and measured by continuous-flow analyzer; dry deposition fluxes were estimated using airborne concentration measurements and inferential models. Our observations reveal large spatial variations of atmospheric Nr concentrations and dry and wet/bulk Nr deposition. On a national basis, the annual average concentrations (1.3-47.0 μg N m-3) and dry plus wet/bulk deposition fluxes (2.9-83.3 kg N ha-1 yr-1) of inorganic Nr species are ranked by land use as urban > rural > background sites and by regions as north China > southeast China > southwest China > northeast China > northwest China > Tibetan Plateau, reflecting the impact of anthropogenic Nr emission. Average dry and wet/bulk N deposition fluxes were 20.6 ± 11.2 (mean ± standard deviation) and 19.3 ± 9.2 kg N ha-1 yr-1 across China, with reduced N deposition dominating both dry and wet/bulk deposition. Our results suggest atmospheric dry N deposition is equally important to wet/bulk N deposition at the national scale. Therefore, both deposition forms should be included when considering the impacts of N deposition on environment and ecosystem health.

相关科学

地球与行星科学
大气科学

文献指纹

地球与环境科学

monitoring network

nitrogen

ecosystem health

dry deposition

gauge

spatial variation

plateau

land use

air

monitoring

method

被引量

期刊度量

Scopus度量

年份 CiteScore SJR SNIP
1996
1997
1998
1999
2000
2001
2002 0.954 0.256
2003 1.199 0.648
2004 2.324 1.133
2005 2.293 1.391
2006 2.836 1.54
2007 3.312 1.747
2008 3.511 1.431
2009 3.781 1.6
2010 3.412 1.51
2011 8.2 3.279 1.484
2012 9.6 3.944 1.574
2013 10.1 3.796 1.811
2014 9.4 3.607 1.681
2015 8.9 3.298 1.522
2016 9.3 3.356 1.783
2017 9.3 3.032 1.546
2018 9.7 2.938 1.662
2019 9.7 2.601 1.517
2020 9.4

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